14.3.2018 Dr. Stephan Thürmer from The University of Kyoto visited us
During his Europe-tour, Stephan Thürmer, very welcomed long-term expat and designer of the previous liquidjet experimental setup, the LiquidjetPES at BESSY, joined us for one day in our commissioning beamtime. As in the good-old times, Stephan got immediately familiar with our new SOL³ system and gave valuable input to improve the lens tables of our hemispherical electron analyzer, pushing the electron transmission to new highs.
13.12.2017 Dr. Alex Gaiduk from The University of Chicago visited us
Our theory collaborator from Giulia Gallis group at ‘UChi’, Alex Gaiduk, visited our group and took a look at our experimental setups at BESSY. He was impressed by the machines that confirm (and on rare occasions ‘readjust’) his invaluable calculated energies and redox potentials from aqueous salt solutions. He also presented his newest ab-initio calculations on one of the hot topics in the water-community: the precise energy position of liquid water’s conduction band - an important number that is experimentally very hard to derive. For more details on Alex work check out his newest article and the Galli group webpage.
13.11.2017 Our article about the iron-(III)-oxo oligomer formation in aqueous solution is online
Together with the research groups of Franziska Emmerling at the BAM Federal Institute for Materials Research and Testing, Berlin, Ralph Krähnert at the Technical University Berlin, and Bernd Winter at Fritz-Haber-Institut der Max-Planck-Gesellschaft, we looked into the formation process of small iron-oxo oligomers in aqueous solution. This chemical process is crucial for the formation of nanoparticles in aqueous phase. By a combination of Raman spectroscopy, Small Angle X-ray scattering and Liquid-microjet resonant photoelectron spectroscopy we could identify and measure the electronic structure properties of the iron-oxo oligomeric seeds that were produced by adding sodium hydroxide to our iron chloride solution. Our findings have been published in Physical Chemistry Chemical Physics. For more details click here.
28.9.2017 First gas dynamic virtual nozzle measurements with our setup
Together with our collaborators from FHI Berlin and IOM Leipzig we successfully measured for the first time at our setup a liquid jet, surrounded by a strong gas-stream to investigate gas-liquid interactions. Claudia, Bernd, and Sebastian from FHI were interested in the CO2 uptake of monoethanolamine in aqueous solutions and looked for its reaction products with respect to the gas-solution interface, and as a function of pH. An exciting experiment!
31.7.2017 Our new SOL³PES setup goes into user operation
Just in time for the start of the user operation of our new SOL³PES setup we got a technical article accepted in Review of Scientific Instruments, describing in detail its capabilities and features. Click here.
19.7.2017 Emmy-Noether meeting in Potsdam
Robert joined the annual three-day meeting as Emmy-Noether-‘freshman’, which took place for the 16th times. This year the current Emmy-Noether stipend holders and alumni met at the lovely Templiner See in Potsdam to talk about funding opportunities, career options after the Emmy-Noether stipend and the changes to the general social conditions in science and politics. For more details check out this DFG site (in German only).
10.4.2017 Beamtime at the U49/2-PGM-1 beamline at BESSY II
This beamtime we further explored metal oxide nanoparticles in water by liquidjet photoelectron spectroscopy. Arno prepared an Fe3O4 nanoparticle solution in our glove box – it is not an easy experiment. Jet stability and concentration are at their limits (and beyond…).
20.3.2017 Beamtime at UE52-SGM-1 beamline at BESSY II
We measured for the first time with our new SOL³PES setup angle-resolved valence photoelectron spectra of neat water. These measurements are key to derive the so-called anisotropy parameter of the outer water valence orbitals. By comparison with gas phase water anisotropy parameter values we can directly determine elastic and inelastic scattering behavior of the outgoing photoelectrons and indirectly the electron mean free path in water – a very important measure for the probing depth. To get our machine to the UE52-SGM-1 beamline we had to use the BESSY crane.
This beamtime was part of the 1st international photonschool at HZB, where 20 international postdocs, master and Phd students got hands-on experience on several experimental BESSY stations, including our SOL³ setup. See more
9.3.2017 Sensitive Method for Detecting Ion Pairs in Aqueous Solutions
Our work on Electron-Transfer Mediated Decay in aqueous solutions was published in Nature Chemistry. See more
1.3.2017 Welcome Arno Bergmann!
Dr. Arno Bergmann, from TU Berlin, joins the team as a postdoctoral research fellow. A very warm welcome!