Schmidt-Mende, L.; Dyakonov, V.; Olthof, S.; Ünlü, F.; Lê, K.M.T.; Mathur, S.; Karabanov, A.D.; Lupascu, D.C.; Herz, L.M.; Hinderhofer, A.; Schreiber, F.; Chernikov, A.; Egger, D.A.; Shargaieva, O.; Cocchi, C.; Unger, E.; Saliba, M.; Byranvand, M.M.; Kroll, M.; Nehm, F.; Leo, K.; Redinger, A.; Höcker, J.; Kirchartz, T.; Warby, J.; Gutierrez-Partida, E.; Neher, D.; Stolterfoht, M.; Würfel, U.; Unmüssig, M.; Herterich, J.; Baretzky, C.; Mohanraj, J.; Thelakkat, M.; Maheu, C.; Jaegermann, W.; Mayer, T.; Rieger, J.; Fauster, T.; Niesner, D.; Yang, F.; Albrecht, S.; Riedl, T.; Fakharuddin, A.; Vasilopoulou, M.; Vaynzof, Y.; Moia, D.; Maier, J.; Franckevicius, M.; Gulbinas, V.; Kerner, R.A.; Zhao, L.; Rand, B.P.; Glück, N.; Bein, T.; Matteocci, F.; Castriotta, L.A.; Di Carlo, A.; Scheffler, M.; Draxl, C.: Roadmap on organic-inorganic hybrid perovskite semiconductors and devices. APL Materials 9 (2021), p. 109202/1-82
10.1063/5.0047616
Open Access Version
Abstract:
Metal halide perovskites are the first solution processed semiconductors that can compete in their functionality with conventional semiconductors, such as silicon. Over the past several years, perovskite semiconductors have reported breakthroughs in various optoelectronic devices, such as solar cells, photodetectors, light emitting and memory devices, and so on. Until now, perovskite semiconductors face challenges regarding their stability, reproducibility, and toxicity. In this Roadmap, we combine the expertise of chemistry, physics, and device engineering from leading experts in the perovskite research community to focus on the fundamental material properties, the fabrication methods, characterization and photophysical properties, perovskite devices, and current challenges in this field. We develop a comprehensive overview of the current state-of-the-art and offer readers an informed perspective of where this field is heading and what challenges we have to overcome to get to successful commercialization.