Dynamics in one-dimensional spin chains newly elucidated

The data from neutron scattering (left) provide information about absorbed energies in reciprocal space. With the new evaluation, it has been possible to obtain statements about new magnetic states and their temporal development in real space (right). The colours blue and red indicate the two opposite spin directions.

The data from neutron scattering (left) provide information about absorbed energies in reciprocal space. With the new evaluation, it has been possible to obtain statements about new magnetic states and their temporal development in real space (right). The colours blue and red indicate the two opposite spin directions. © HZB

Neutron scattering is considered the method of choice for investigating magnetic structures and excitations in quantum materials. Now, for the first time, the evaluation of measurement data from the 2000s with new methods has provided much deeper insights into a model system – the 1D Heisenberg spin chains. A new toolbox is available for elucidating future quantum materials has been achieved.

Potassium copper fluoride KCuF3 is considered the simplest model material realising the so-called Heisenberg quantum spin chain: The spins interact with their neighbours antiferromagnetically along a single direction (one-dimensional), governed by the laws of quantum physics.

"We carried out the measurements on this simple model material at the ISIS spallation neutron source some time ago when I was a postdoc, and we  published our results in 2005, 2013 and again in 2021 comparing to new theories each time they became available," says Prof. Bella Lake, who heads the HZB-Institute Quantum Phenomena in Novel Materials. Now with new and extended methods, a team led by Prof. Alan Tennant and Dr Allen Scheie have succeeded to gain significantly deeper insights into the interactions between the spins and their spatial and temporal evolution.

Dynamics like a wake

"With neutron scattering, you sort of nudge a spin so that it flips. This creates a dynamic, like a wake when a ship is sailing through water, which can affect its neighbours and their neighbours," Tennant explains.

”Neutron scattering data is measured as a function of energy and wavevector” says Scheie “ Our breakthrough was to map the spatial and temporal development of the spins using mathematical methods such as a back-Fourier transformation.” Combined with other theoretical methods, the physicists gathered information about interactions between the spin states and their duration and range, as well as insights into the so-called quantum coherence.

New tool box

The work demonstrates a new tool box for the analysis of neutron scattering data and might foster a deeper understanding of quantum materials that are relevant for technological use.

arö

  • Copy link

You might also be interested in

  • HZB and National University Kyiv-Mohyla Academy start cooperation in Energy and Climate
    News
    19.06.2025
    HZB and National University Kyiv-Mohyla Academy start cooperation in Energy and Climate
    Helmholtz-Zentrum Berlin für Materialien und Energie GmbH (HZB) and the National University of "Kyiv-Mohyla Academy" (NaUKMA) have signed a Memorandum of Understanding (MoU). The MoU serves as the starting point for collaborative research, academic exchange, and capacity-building between the two institutions. Actions will be taken to establish the Joint Research and Policy Laboratory at NaUKMA in Kyiv. The aim of the future laboratory is to jointly develop research and policy analysis, focusing on the energy and climate dimensions of Ukraine’s EU integration.
  • MAX IV and BESSY II initiate new collaboration to advance materials science
    News
    17.06.2025
    MAX IV and BESSY II initiate new collaboration to advance materials science
    Swedish national synchrotron laboratory MAX IV and Helmholtz-Zentrum Berlin (HZB) with BESSY II light source jointly announce the signing of a 5-year Cooperation Agreement. The new agreement establishes a framework to strengthen cooperation for operational and technological development in the highlighted fields of accelerator research and development, beamlines and optics, endstations and sample environments as well as digitalisation and data science.
  • Michael Naguib is visiting HZB as a Humboldt Research Awardee
    News
    16.06.2025
    Michael Naguib is visiting HZB as a Humboldt Research Awardee
    Professor Michael Naguib, from Tulane University in the USA, is one of the discoverers of a new class of 2D materials: MXenes are characterised by a puff pastry-like structure and have many applications, such as in the production of green hydrogen or as storage media for electrical energy. During his Humboldt Research Award in 2025, Professor Naguib is working with Prof Volker Presser at the Leibniz Institute for New Materials in Saarbrücken and with Dr Tristan Petit at HZB.