Emergence of a “devil’s staircase” in a spin-valve system
Hexagonal single crystal of SrCo6O11, with a sample diameter of approximately 0,2 millimetres.
The material exhibits distinct magnetization plateau connected with different spin configurations.
A Japanese-German team observes at BESSY II how spins form unusual magnetic structures in a complex cobalt oxide single crystal. Such a material offers new perspectives for spintronic applications.
While classical GMR systems are composed of metallic layers, complex oxides often intrinsically provide layered structures with alternating magnetic configurations that can act as spin valves. Cobalt oxides are a class of materials that can exhibit complex magnetic order that changes with increasing magnetic field, as for example indicated by distinct plateaux in the magnetization curve.
Magnetic structures mapped
A Japanese team of researchers led by the group of Associate Professor Hiroki Wadati at the University of Tokyo has been successful in characterizing the magnetic structures of the complex cobalt oxide SrCo6O11 using the high-field diffractometer of BESSY II. Synthesis of new materials often results in tiny samples, and the crystals studied here had a diameter of only 0.2 mm. With the very high sensitivity of resonant diffraction, a core competence at the UE46_PGM1 beamline of BESSY II, they managed to observe a fascinating type of spin order in the samples that are hardly visible by the bare eye. This order is called devil’s staircase, characterizing a phenomenon, where a pletora, in principle even an infinite number, of so-called commensurate superstructures - magnetic configurations in the present case - can be realized by tuning an external parameter, e.g., a magnetic field.
New options with a Devil's staircase
This exceeds the characteristic of a spin valve and may open new paths in spintronics. The research was carried out in close cooperation with German scientists from the Institut für Festkörper-und Werkstoffforschung Dresden and HZB. The results are now published in Physical Review Letters.
Reference: T. Matsuda, S. Partzsch, T. Tsuyama, E. Schierle, E. Weschke, J. Geck, T. Saito, S. Ishiwata, Y. Tokura, and H. Wadati, "Observation of a Devil’s Staircase in the Novel Spin-Valve System SrCo6O11", Physical Review Letters 114 (236403-1-5):
doi:10.1103/PhysRevLett.114.236403.
- BESSY II: Phosphorous chains – a 1D material with 1D electronic propertiesFor the first time, a team at BESSY II has succeeded in demonstrating the one-dimensional electronic properties of a material through a highly refined experimental process. The samples consisted of short chains of phosphorus atoms that self-organise at specific angles on a silver substrate. Through sophisticated analysis, the team was able to disentangle the contributions of these differently aligned chains. This revealed that the electronic properties of each chain are indeed one-dimensional. Calculations predict an exciting phase transition to be expected as soon as these chains are more closely packed. While material consisting of individual chains with longer distances is semiconducting, a very dense chain structure would be metallic.
- Did marine life in the palaeocene use a compass?Some ancient marine organisms produced mysterious magnetic particles of unusually large size, which can now be found as fossils in marine sediments. An international team has succeeded in mapping the magnetic domains on one of such ‘giant magnetofossils’ using a sophisticated method at the Diamond X-ray source. Their analysis shows that these particles could have allowed these organisms to sense tiny variations in both the direction and intensity of the Earth’s magnetic field, enabling them to geolocate themselves and navigate across the ocean. The method offers a powerful tool for magnetically testing whether putative biological iron oxide particles in Mars samples have a biogenic origin.
- What vibrating molecules might reveal about cell biologyInfrared vibrational spectroscopy at BESSY II can be used to create high-resolution maps of molecules inside live cells and cell organelles in native aqueous environment, according to a new study by a team from HZB and Humboldt University in Berlin. Nano-IR spectroscopy with s-SNOM at the IRIS beamline is now suitable for examining tiny biological samples in liquid medium in the nanometre range and generating infrared images of molecular vibrations with nanometre resolution. It is even possible to obtain 3D information. To test the method, the team grew fibroblasts on a highly transparent SiC membrane and examined them in vivo. This method will provide new insights into cell biology.