SMART
Spectro-Microscopy with aberration correction for relevant techniques
Publikationen
2024de Souza Caldas, L.; Prieto, M.J.; Tanase, L.C.; Tiwari, A.; Schmidt, Th.; Roldan Cuenya, B.: Correlative in situ Spectro-microscopy of Supported Single CuO Nanoparticles: Unveiling the Relationships between Morphology and Chemical State during Thermal Reduction. , ACS Nano 18 (2024), p. 13714-13725
doi: 10.1021/acsnano.4c01460
Prieto, M.J.; de Souza Caldas, L.; Tanase, L.C.; Schmidt, T.; Rodriguez de la Fuente, O.: Spectromicroscopic study of the transformation with low energy ions of a hematite thin film into a magnetite/hematite epitaxial bilayer. , Ultramicroscopy 255 (2024), p. 113855/1-7
doi: 10.1016/j.ultramic.2023.113855
2023
Fuhrich, A.; Paier, J.; Tosoni, S.; Lewandowski, A.L.; Gura, L.; Schneider, W.D.; Pacchioni, G.; Freund, H.-J.: Mixed Germania-Silica Films on Ru(0001): A combined experimental and theoretical study. , Israel Journal of Chemistry 63 (2023), p. e202300005/1-13
doi: 10.1002/ijch.202300005
Pozarowska, E.; Pleines, L; Prieto, M.J.; Ewert, M.; Tanase, L.C.; de Souza Caldas, L.; Tiwari, A.; Schmidt, Th.; Falta, J.; Krasovskii, E.; Flege, J.I.; Morales, C.: Preparation and stability of hexagonal phase of samarium oxide on Ru(0001). , Ultramicroscopy 250 (2023), p. 113755
doi: 10.1016/j.ultramic.2023.113755
Abramiuc, L.E.; Tanase, L.C.; Prieto, M.J.; de Souza Caldas, L.; Tiwari, A.; Apostol, N.G.; Husanu, M.A.; Chirila, C.F.; Trupina, L.; Schmidt, T.; Pintilie, L.; Teodorescu, C.M.: Surface charge dynamics on air-exposed ferroelectric Pb(Zr,Ti)O3(001) thin films. , Nanoscale 15 (2023), p. 13062-13075
doi: 10.1039/d3nr02690f
2022
Pechmann, Sabrina: Molecular adsorbates on epitaxial MgO/Ag(100). , FAU Erlangen, 2022
Michalak, N.; Ossowski, T.; Milosz, Z.; Prieto, M.J.; Wang, Y.; Werwinski, M.; Babacic, V.; Genuzio, F.; Vattuone, L.; Kiejna, A.; Schmidt, T.; Lewandowski, M.: Ostwald Ripening in an Oxide-on-Metal System. , Advanced Materials Interfaces 9 (2022), p. 2200222/1-7
doi: 10.1002/admi.202200222
Zeininger, J.; Winkler, Ph.; Raab, M.; Suchorski, Y.; Prieto, M.J.; Tanase, L.C.; de Souza Caldas, L.; Tiwari, A.; Schmidt, Th.; Stöger-Pollach, M.; Steiger-Thirsfeld, A.; Roldan Cuenya, B.; Rupprechter, G.: Pattern formation in catalytic H2 oxidation on Rh: Zooming in by correlative microscopy. , ACS Catalysis 12 (2022), p. 11974-11983
doi: 10.1021/acscatal.2c03692
Prieto, M.J.; Mullan, Th.; Wan, W.; nase, L.; de Souza Caldas, L.C.; Shaikhutdinov, S.; Sauer, J.; Usvyat, D.; Schmidt, Th.; Roldan Cuenya, B.: Plasma functionalization of silica bilayer polymorphs. , ACS Applied Materials & Interfaces 14 (2022), p. 48609-48618
doi: 10.1021/acsami.2c11491
2021
Rost, H.I.; Reed, B.P.; Strand, F.S.; Durk, J.; Evans, D.A.; Grubisic-Cabo, A.; Wan, G.; Cattelan, M.; Prieto, M.J.; Gottlob, D.M.; Tanase, L.C.; de Souza Caldas, L.; Schmidt, Th.; Tadich, A.; Cowie, B.C.C.; Kumar Chellappan, R.; Cooil, S.P.; Wells, J.W.: A Simplified Method for Patterning Graphene on Dielectric Layers. , ACS Applied Materials & Interfaces 13 (2021), p. 375510-37516
doi: 10.1021/acsami.1c09987
Homann, M.; von Boehn, B.; Prieto, M.J.; Gottlob, D.M.; Tanase, L.C.; Schmidt, Th.; Genuzio, F.; Locatelli, A.; Imbihl, R.: Coupling of morphological instability and kinetic instability: Chemical waves in hydrogen oxidation on a bimetallic Ni/Rh(111) surface. , Physical Review Materials 5 (2021), p. 045002/1-5
doi: 10.1103/PhysRevMaterials.5.045002
Lewandowski, A.L.; Tosoni, S.; Gura, L.; Yang, Z.; Fuhrich, A.; Prieto, M.J.; Schmidt, T.; Usvyat, D.; Schneider, W.D.; Heyde, M.; Pacchioni, G.; Freund, H.J.: Growth and Atomic-Scale Characterization of Ultrathin Silica and Germania Films: The Crucial Role of the Metal Support. , Chemistry - A European Journal 27 (2021), p. 1870-1885
doi: 10.1002/chem.202001806
Prieto, M.J.; Mullan, T.; Schlutow, M.; Gottlob, D.M.; Tanase, L.C.; Menzel, D.; Sauer, J.; Usvyat, D.; Schmidt, T.; Freund, H.J.: Insights into Reaction Kinetics in Confined Space: Real Time Observation of Water Formation under a Silica Cover. , Journal of the American Chemical Society 143 (2021), p. 8780-8790
doi: 10.1021/jacs.1c03197
Rost, H.I.; Chellappan, R.K.; Strand, F.S.; Grubisic-Cabo, A.; Reed, B.P.; Prieto, M.J.; Tanase, L.C.; De Souza Caldas, L.; Wongpinij, T.; Euaruksakul, C.; Schmidt, T.; Tadich, A.; Cowie, B.C.C.; Li, Z.; Cooil, S.P.; Wells, J.W.: Low-Temperature Growth of Graphene on a Semiconductor. , The Journal of Physical Chemistry C 125 (2021), p. 4243-4252
doi: 10.1021/acs.jpcc.0c10870
Kunze, S.; Tanase, L.C.; Prieto, M.J.; Grosse, P.; Scholten, F.; de Souza Caldas, L.; van Voerden, D.; Schmidt, T.; Roldan Cuenya, B.: Plasma-assisted oxidation of Cu(100) and Cu(111). , Chemical Science 12 (2021), p. 14241-14253
doi: 10.1039/d1sc04861a
2020
Freund, H.-J.; Heyde, M.; Kuhlenbeck, H.; Nilius, N.; Risse, T.; Schmidt, T.; Shaikhutdinov, S.; Sterrer, M.: Chapter model systems in heterogeneous catalysis at the atomic level: a personal view. , Science China = Scientia Sinica. Chemistry 63 (2020), p. 426-447
doi: 10.1007/s11426-019-9671-0
Schweinar, K.; Beeg, S.; Hartwig, C.; Rajamathi, C.R.; Kasian, O.; Piccinin, S.; Prieto, M.J.; Tanase, L.C.; Gottlob, D.M.; Schmidt, T.; Raabe, D.; Schlögl, R.; Gault, G.; Jones, T.E.; Greiner, M.T.: Formation of a 2D Meta-stable Oxide by Differential Oxidation of AgCu Alloys. , ACS Applied Materials & Interfaces 12 (2020), p. 23595–23605
doi: 10.1021/acsami.0c03963
Silvestri, F.; Prieto, M.J.; Tanase, L.C.; de Souza Caldas, L.; Tessler, N.; Solomeshch, O.; Schmidt, Th.; Ocal, C.; Barrena, E.: Impact of thin film structure on the pentance-C60F48 interface formation and charge transfer. , ACS Applied Materials & Interfaces 12 (2020), p. 25444-25452
doi: 10.1021/acsami.0c05583
Klemm, H.W.; Prieto, M.J.; Xiong, F.; Hassine, G.B.; Heyde, M.; Menzel, D.; Sierka, M.; Schmidt, Th.; Freund, H.-J.: Silica bilayer supported on Ru(0001): Following the crystalline to vitreous transformation in real time with spectro-microscopy. , Angewandte Chemie - International Edition 59 (2020), p. 10587–10593
doi: 10.1002/anie.202002514
2019
Schmidt, T.; Marchetto, H.; Groh, U.; Fink, R.H.; Umbach, E.: Complex monolayer growth dynamics of a highly symmetric molecule: NTCDA on Ag(111). , The Journal of Physical Chemistry C 123 (2019), p. 8244-8255
doi: 10.1021/acs.jpcc.8b08523
Mor, Selene: Fundamental interactions governing the (non-)equilibrium electronic structure in low dimensions. , Berlin, Freie Universität Berlin, Diss., 2019
Fuhrich, Alexander Benedikt: Ultra-thin Germania and Germania-Silica films : growth, structure and reactivity. , Berlin, Freie Universität Berlin, Diss., 2019
2018
Kuhness, D.; Yang, H.J.; Klemm, H.W.; Prieto, M.; Peschel, G.; Fuhrich, A.; Menzel, D.; Schmidt, T.; Yu, X.; Shaikhutdinov, S.; Lewandowski, A.; Heyde, M.; Kelemen, A.; Wlodarczyk, R.; Usvyat, D.; Schutz, M.; Sauer, J.; Freund, H.J.: A Two-Dimensional 'Zigzag' Silica Polymorph on a Metal Support. , Journal of the American Chemical Society 140 (2018), p. 6164-6168
doi: 10.1021/jacs.8b02905
Klemm, H.W.; Prieto, M.J.; Peschel, G.; Fuhrich, A.; Madej, E.; Xiong, F.; Menzel, D.; Schmidt, Th.; Freund, H.-J.: Formation and Evolution of Ultrathin Silica Polymorphs on Ru(0001) Studied With Combined in Situ, Real-Time Methods. , The Journal of Physical Chemistry C 123 (2018), p. 8228-8243
doi: 10.1021/acs.jpcc.8b08525
Klemm, Hagen William: Formation and properties of ultrathin silicon dioxide films on Ru(0001). , Berlin, Technische Universität, Diss., 2018
Peschel, Gina: Growth and structure of ultrathin silicates and germanates containing iron oxide. , Berlin, Freie Universität Berlin, Diss., 2018
Schmidt, T.; Marchetto, H.; Groh, U.; Fink, R.H.; Freund, H.J.; Umbach, E.: Influence of Substrate Bonding and Surface Morphology on Dynamic Organic Layer Growth: Perylenetetracarboxylic Dianhydride on Au(111). , Langmuir 34 (2018), p. 5444-5453
doi: 10.1021/acs.langmuir.8b00493
Hartmann, C.; Sadoughi, G.; Felix, R.; Handick, E.; Klemm, H.W.; Peschel, G.; Madej, E.; Fuhrich, A.B.; Liao, X.; Raoux, S.; Abou-Ras, D.; Wargulski, D.; Schmidt, Th.; Wilks, R.G.; Snaith, H.; Bär, M.: Spatially-resolved insight into the chemical and electronic structure of solution processed perovskites – why to (not) worry about pin-holes. , Advanced Materials Interfaces 5 (2018), p. 1701420/1-9
doi: 10.1002/admi.201701420
Michalak, N.; Milosz, Z.; Peschel, G.; Prieto, M.; Xiong, F.; Wojciechowski, P.; Schmidt, Th.; Lewandowski, M.: Symmetry-induced structuring of ultrathin FeO and Fe3O4 films on Pt(111) and Ru(0001). , Nanomaterials 8 (2018), p. 719/1-14
doi: 10.3390/nano8090719
Prieto, M.J.; Klemm, H.W.; Xiong, F.; Gottlob, D.M.; Menzel, D.; Schmidt, T.; Freund, H.-J.: Wasserbildung unter dünnen Silika-Filmen: Echtzeitbeobachtung einer chemischen Reaktion in einem physikalisch eingegrenzten Raum. , Angewandte Chemie 130 (2018), p. 8885-8889
doi: 10.1002/ange.201802000
Prieto, M.J.; Klemm, H.W.; Xiong, F.; Gottlob, D.M.; Menzel, D.; Schmidt, T.; Freund, H.-J.: Water Formation under Silica Thin Films: Real-Time Observation of a Chemical Reaction in a Physically Confined Space. , Angewandte Chemie - International Edition 57 (2018), p. 8749-8753
doi: 10.1002/anie.201802000
2017
Breuer, T.; Karthauser, A.; Klemm, H.W.; Genuzio, F.; Peschel, G.; Fuhrich, A.; Schmidt, T.; Witte, G.: Exceptional Dewetting of Organic Semiconductor Films: the Case of Dinaphthothienothiophene (DNTT) at Dielectric Interfaces. , ACS Applied Materials & Interfaces 9 (2017), p. 8384-8392
doi: 10.1021/acsami.6b15902
Cooil, S.P.; Mazzola, F.; Klemm, H.W.; Peschel, G.; Niu, Y.R.; Zakharov, A.A.; Simmons, M.Y.; Schmidt, T.; Evans, D.A.; Miwa, J.A.; Wells, J.W.: In Situ Patterning of Ultrasharp Dopant Profiles in Silicon. , ACS Nano 11 (2017), p. 1683-1688
doi: 10.1021/acsnano.6b07359
Eylers, K.; Ringleb, F.; Heidmann, B.; Levcenco, S.; Unold, T.; Klemm, H.W.; Peschel, G.; Fuhrich, A.; Teubner, T.; Schmidt, T.; Schmid, M.; Boeck, T.: In-Ga precursor islands for Cu(In,Ga)Se2 micro-concentrator solar cells. , In: Get energized with solar power : 44th IEEE Photovoltaic Specialists Conference, Washington, DC, June 25-30, 2017Piscataway, NJ: IEEE, 2017. - ISBN 978-1-5090-5606-4, p. 3396-3401
doi: 10.1109/PVSC.2017.8366526
Schulz, K.; Schmack, R.; Klemm, H.W.; Kabelitz, A.; Schmidt, T.; Emmerling, F.; Kraehnert, R.: Mechanism and Kinetics of Hematite Crystallization in Air: Linking Bulk and Surface Models via Mesoporous Films with Defined Nanostructure. , Chemistry of Materials 29 (2017), p. 1724-1734
doi: 10.1021/acs.chemmater.6b05185
Pollinger, P.; Schmitt, S.; Sander, D.; Tian, Z.; Kirschner, J.; Vrdoljak, P.; Stadler, C.; Maier, F.; Marchetto, H.; Schmidt, T.; Schöll, A.; Umbach, E.: Nanoscale patterning, macroscopic reconstruction, and enhanced surface stress by organic adsorption on vicinal surfaces. , New Journal of Physics 19 (2017), p. 013019/1-12
doi: 10.1088/1367-2630/aa55b8
Tinti, G.; Marchetto, H.; Vaz, C.A.F.; Kleibert, A.; Andrä, M.; Barten, R.; Bergamaschi, A.; Brücker, M.; Cartier, S.; Dinapoli, R.; Franz, T.; Fröjdh, E.; Greiffenberg, D.; Lopez-Cuenca, C.; Mezza, D.; Mozzanica, A.; Nolting, F.; Ramilli, M.; Redford, S.; Ruat, M.; Ruder, Ch.; Schädler, L.; Schmidt, Th.; Schmitt, B.; Schutz, F.; Shi, X.; Thattil, D.; Vetter, S.; Zhang, J.: The EIGER detector for low-energy electron microscopy and photoemission electron microscopy. , Journal of Synchrotron Radiation 24 (2017), p. 963-974
doi: 10.1107/S1600577517009109
2016
Lévesque, P.L.; Marchetto, H.; Schmidt, Th.; Maier, F.C.; Freund, H.-J.; Umbach, E: Correlation between substrate morphology and the initial stages of epitaxial organic growth – PTCDA/Ag(111). , The Journal of Physical Chemistry C 120 (2016), p. 19271–19279
doi: 10.1021/acs.jpcc.6b06781
Genuzio, F.; Sala, A.; Schmidt, Th.; Menzel, D.; Freund, H.-J.: Phase transformations in thin iron oxide films: Spectromicroscopic study of velocity and shape of the reaction fronts. , Surface Science 648 (2016), p. 177–187
doi: 10.1016/j.susc.2015.11.016
Genuzio, Francesca: Spectro-microscopic investigation of Fe-oxide based model catalysts and instrumental development. , Berlin, Humboldt Universität, Diss., 2016
Cooil, S.P.; Mortsell, E.A.; Mazzola, F.; Jorge, M.; Wenner, S.; Edmonds, M.T.; Thomsen, L.; Klemm, H.W.; Peschel, G.; Fuhrich, A.; Prieto, M.; Schmidt, Th.; Miwa, J.A.; Holmestad, R.; Wells, J.W.: Thermal migration of alloying agents in aluminium. , Materials Research Express 3 (2016), p. 116501/1-8
doi: 10.1088/2053-1591/3/11/116501
2015
Marchetto, H.; Schmidt, Th.; Groh, U.; Maier, F.C.; Lévesque, P.L.; Fink, R.H.; Freund, H.-J.; Umbach, E.: Direct observation of epitaxial organic film growth: temperature-dependent growth mechanisms and metastability. , Physical Chemistry Chemical Physics 17 (2015), p. 29150-29160
doi: 10.1039/C5CP05124J
Casu, M.B.: Growth, structure, and electronic properties in organic thin films deposited on metal surfaces investigated by low energy electron microscopy and photoelectron emission microscopy. , Journal of Electron Spectroscopy and Related Phenomena 204 (2015), p. 39-48
doi: 10.1016/j.elspec.2015.03.001
Klemm, H.W.; Peschel, G.; Madej, E.; Fuhrich, A.; Timm, M.; Menzel, D.; Schmidt, Th.; Freund, H.-J.: Preparation of Silica Films on Ru(0001): a LEEM/PEEM Study. , Surface Science 643 (2015), p. 45-51
doi: 10.1016/j.susc.2015.05.017
2014
Genuzio, F.; Sala, A.; Schmidt, Th.; Menzel, D.; Freund, H.-J.: Interconversion of α-Fe2O3 and Fe3O4 Thin Films: Mechanisms, Morphology, and Evidence for Unexpected Substrate Participation. , The Journal of Physical Chemistry C 118 (2014), p. 29068-29076
doi: 10.1021/jp504020a
2013
Sala, Alessandro: Characterization of iron oxide thin films as a support for catalytically active nanoparticles. , Berlin, Freie Universität Berlin, Diss., 2013
Schmidt, T.; Sala, A.; Marchetto, H.; Umbach, E.; Freund, H.-J.: First experimental proof for aberration correction in XPEEM: Resolution, transmission enhancement, and limitation by space charge effects. , Ultramicroscopy 126 (2013), p. 23-32
doi: 10.1016/j.ultramic.2012.11.004
2012
Sala, A.; Marchetto, H.; Qin, Z.-H.; Shaikhutdinov, S.; Schmidt, Th.; Freund, H.-J.: Defects and inhomogeneities in Fe3O4(111) thin film growth on Pt(111). , Physical Review B 86 (2012), p. 155430/1-10
doi: 10.1103/PhysRevB.86.155430
Casu, M.B.; Savu, S.-A.; Schuster, B.-E.; Biswas, I.; Raisch, C.; Marchetto, H.; Schmidt, Th.; Chasse, T.: Island shapes and aggregation steered by the geometry of the substrate lattice. , Chemical Communications 48 (2012), p. 6957-6959
doi: 10.1039/c2cc31339A
2011
Freund, H.-J.; Nilius, N.; Risse, T.; Schauermann, S.; Schmidt, T.: Innovative Measurement Techniques in Surface Science. , ChemPhysChem 12 (2011), p. 79-87
doi: 10.1002/cphc.201000812
2010
Schmidt, Th.; Marchetto, H.; Levesque, P.L.; Groh, U.; Maier, F.; Preikszas, D.; Hartel, P.; Spehr, R.; Lilienkamp, G.; Engel, W.; Fink, R.; Bauer, E.; Rose, H.; Umbach, E.; Freund, H.-J.: Double aberration correction in a low-energy electron microscope. , Ultramicroscopy 110 (2010), p. 1358-1361
doi: 10.1016/j.ultramic.2010.07.007
Casu, M.B.; Schuster, B.E.; Biswas, I.; Raisch, C.; Marchetto, H.; Schmidt, T.; Chassé, T.: Locally resolved core-hole screening, molecular orientation, and morphology in thin films of diindenoperylene deposited on Au(111) single crystals. , Advanced Materials 22 (2010), p. 3740-3744
doi: 10.1002/adma.201001265
Maier, Florian C.: Spectromicroscopic characterisation of the formation of complex interfaces. , Würzburg, Universität Würzburg, Diss., 2010
2009
Pollinger, Florian: Surface stress and large-scale self-organization at organic-metal interfaces. , Diss., Univ. Würzburg, 2009
SMART