First Observation of Undulator Photon Beams Carrying Orbital Angular Momentum

The measurement (left) is impressively well reproduced in a simulation utilizing the HZB-code WAVE.

The measurement (left) is impressively well reproduced in a simulation utilizing the HZB-code WAVE. © J. Bahrdt/HZB

For the first time researchers of HZB observed 99eV photons carrying Orbital Angular Momentum (OAM). The photons were detected in the 2nd harmonic off-axis radiation of a helical undulator. The measurements confirm a theoretical prediction from five years ago. In the visible regime these singular photon beams or OAM-photons can be generated from laser light utilizing phase modulating techniques. The proof-of-principle experiment at BESSY II demonstrates the availability of OAM-photons up to the X-ray regime in low emittance machines, with helical undulators being used for the generation of circularly polarized radiation similar to today’s 3rd generation light sources.

Under normal operation conditions – electron energy of 1.72 GeV - the BESSY II beam emittance (i.e. the electron bunch phase space volume) is too large for the detection of the singular phase structure of OAM-photons. The emittance scales quadratically with the energy, and, thus, at 917 MeV (energy of a former PTB- electron optic) the emittance is reduced roughly by a factor of four which is sufficient for a clear well-defined experiment.  In January 2013 the BESSY II storage ring was ramped down for a 24h shift from 1.72 GeV to 917 MeV. An injection at 917 MeV was not possible and, hence, all storage ring magnets had to be tuned simultaneously during this delicate procedure in order minimize electron losses.

The interference experiment with the double undulator UE56-2 was conducted by a team around Dr. Johannes Bahrdt. One undulator was tuned to helical mode generating OAM photons in the 2nd harmonic. The other undulator served as a reference undulator providing linearly polarized light. The transverse distribution of both photon beams was mapped with a pinhole in front of the 1st optical element. The longitudinal overlap and the interference happened only behind the monochromator. The direct detection of the singular phase distribution of OAM beams would require a complicated wavefront sensor whereas the interference experiment permitted an intensity detection with a simple diode. The signature of the OAMs is a spiral intensity distribution where the orientation is determined by the helicity of the helical undulator and the spiral orientation is a measure of the phase advance between both undulators.

The joint effort of people from several HZB-groups (P. Kuske, P. Schmid: G-IA; R. Müller: NP-ABS, K. Holldack: G-ISRR and J. Bahrdt, M. Scheer: G-AUND) resulted in the success of this experiment, particularly, because it required specific machine conditions and the beam current was only 1mA. Photons carrying orbital angular momentum will be available permanently in synchrotron radiation light sources of the next generation such as Energy Recovery Linacs, Ultimate Storage Rings or Free Electron Lasers. The additional degree of freedom may trigger new spectroscopic experiments which are not possible at existing light sources.

Physical Review Letters (DOI: 10.1103/PhysRevLett.111.034801)

hs

  • Copy link

You might also be interested in

  • Spin waves inside a nano-oscillator imaged for the first time
    Science Highlight
    23.09.2026
    Spin waves inside a nano-oscillator imaged for the first time
    For the first time, researchers have directly imaged the magnetisation dynamics inside a spin Hall nano-oscillator — a nanoscale device that converts direct current into tunable microwave signals and is a promising building block for energy-efficient wireless communication and brain-inspired computing. A Swedish–German team led by the University of Gothenburg and Helmholtz-Zentrum Berlin (HZB) achieved this using time-resolved scanning transmission X-ray microscopy at the MAXYMUS instrument at BESSY II. The results, now published in Advanced Materials, reveal spin-wave features that had escaped previous, indirect measurement techniques.
  • BESSY II: High-resolution insights into individual biomolecules and catalysts
    Science Highlight
    15.09.2026
    BESSY II: High-resolution insights into individual biomolecules and catalysts
    Very small biological samples and even individual biomolecules can now be examined under near-physiological conditions with high confidence at the BESSY II infrared beamline with a newly validated and improved technique: The nanoscale infrared spectroscopy (s-SNOM) with ultra-thin silicon-based membranes. An international team demonstrated after an initial proof of concept, that high-resolution (a few tens of nanometres) nano-IR measurements reliably match expected far-field IR spectra in an aqueous environment. This methodological advance provides a solid foundation for studying biomaterials or observing catalytic processes in a liquid environment.
  • New method shows how molecular switches are influenced by their neighbors
    Science Highlight
    11.09.2026
    New method shows how molecular switches are influenced by their neighbors
    Researchers at Friedrich Schiller University Jena and the Helmholtz Centre Berlin (HZB) have, for the first time, been able to directly observe how the environment surrounding a molecular switch influences its electronic structure. Molecular switches are molecules that can be switched between two states by external influences such as changes in temperature—similar to a switch with the positions »On« and »Off«. Such molecules are being investigated as potential building blocks for future data storage devices or sensor materials. Using magnetic-field-dependent terahertz spectroscopy, the researchers have now, for the first time, been able to distinguish whether neighbouring molecules in a material are in the same or different states. The results have been published in the journal »Angewandte Chemie International Edition«.